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Polyethylene terephthalate is a valuable commercial product useful as fibers or resins in such products as carpets and synthetic fibers. It is a useful monomer for the production of a variety of useful polymers including, but not limited to, polyesters, polyamides, polycarbonates, polyetherimides, and polyetheretherketones.
Use of polyethylene terephthalate as a fiber has been increased in recent years because of its combination of good properties of heat resistance, chemical resistance, etc. However, it has the drawback of a poor property of biodegradability.
The conventional process for the production of polyethylene terephthalate has been realized by two different methods. One is the esterification process of terephthalic acid or its reactive derivative (e.g. dimethyl terephthalate) with ethylene glycol followed by polycondensation, and the other is direct polymerization of ethylene terephthalate or its reactive derivative (e.g. ethylene dimethyl terephthalate).
The esterification process of terephthalic acid or its reactive derivative with ethylene glycol cannot be carried out at a high reaction temperature for a long time because the acid or the reactive derivative decomposes or hydrolyzes during the esterification reaction.
It has been proposed to use terephthalic acid or its reactive derivative as an esterification agent to avoid such hydrolysis (see, U.S. Pat. No. 5,120,869 and EP Patent Application No. 81307756.1). However, the reaction proceeds under mild conditions and produces a polyester by a solid phase reaction, and it is very difficult to control the molecular weight of the polyester product.
On the other hand, in the process of direct polymerization

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